He was the Portuguese First Division's top scorer seven times (1964, 1965, 1966, 1967, 1968, 1970 and 1973), helping Benfica to win 11 Primeira Liga (1960–61, 1962–63, 1963–64, 1964–65, 1966–67, 1967–68, 1968–69, 1970–71, 1971–72, 1972–73 and 1974–75), 5 Portuguese Cup wins (1961–62, 1963–64, 1968–69, 1969–70 and 1971–72), 1 European Cup win (1961–62) and 3 European Cup finals (1962–63, 1964–65 and 1967–68).
Foi melhor marcador da Primeira Divisão portuguesa sete vezes (1964, 1965, 1966, 1967, 1968, 1970 e 1973), ajudando o Benfica a ser 11 vezes o campeão da Primeira Divisão (1960–61, 1962–63, 1963–64, 1964–65, 1966–67, 1967–68, 1968–69, 1970–71, 1971–72, 1972–73 e 1974–75), vencer 5 vezes a Taça de Portugal (1961–62, 1963–64, 1968–69, 1969–70 e 1971–72), uma vez a Taça dos Campeões Europeus (1961–62) e três vezes finalista da Taça dos Campeões Europeus (1962–63, 1964–65 e 1967–68).