  Electron-phonon coupling directly determines the stability of cooperative
order in solids, including superconductivity, charge and spin density waves.
Therefore, the ability to enhance or reduce electron-phonon coupling by optical
driving may open up new possibilities to steer materials' functionalities,
potentially at high speeds. Here we explore the response of bilayer graphene to
dynamical modulation of the lattice, achieved by driving optically-active
in-plane bond stretching vibrations with femtosecond mid-infrared pulses. The
driven state is studied by two different ultrafast spectroscopic techniques.
Firstly, TeraHertz time-domain spectroscopy reveals that the Drude scattering
rate decreases upon driving. Secondly, the relaxation rate of hot
quasi-particles, as measured by time- and angle-resolved photoemission
spectroscopy, increases. These two independent observations are quantitatively
consistent with one another and can be explained by a transient three-fold
enhancement of the electron-phonon coupling constant. The findings reported
here provide useful perspective for related experiments, which reported the
enhancement of superconductivity in alkali-doped fullerites when a similar
phonon mode was driven.
