  Realizing a large Land\'{e} $g$-factor of electrons in solid-state materials
has long been thought of as a rewarding task as it can trigger abundant
immediate applications in spintronics and quantum computing. Here, by using
metamorphic InAsSb/InSb superlattices (SLs), we demonstrate an unprecedented
high value of $g\approx 104$, twice larger than that in bulk InSb, and fully
spin-polarized states at low magnetic fields. In addition, we show that the
$g$-factor can be tuned on demand from 20 to 110 via varying the SL period. The
key ingredients of such a wide tunability are the wavefunction mixing and
overlap between the electron and hole states, which have drawn little attention
in prior studies. Our work not only establishes metamorphic InAsSb/InSb as a
promising and competitive material platform for future quantum devices but also
provides a new route toward $g$-factor engineering in semiconductor structures.
