  Gravitational waves with frequencies below 1~nHz are notoriously difficult to
detect. With periods exceeding current experimental lifetimes, they induce slow
drifts in observables rather than periodic correlations. Observables with
well-known intrinsic contributions provide a means to probe this regime. In
this work, we demonstrate the viability of using observed pulsar timing
parameters to discover such "ultralow" frequency gravitational waves,
presenting two complementary observables for which the systematic shift induced
by ultralow-frequency gravitational waves can be extracted. Using existing data
for these parameters, we search the ultralow frequency regime for
continuous-wave signals, finding a sensitivity near the expected prediction
from inspirals of supermassive black holes. We do not see an excess in the
data, setting a limit on the strain of $ 1.3 \times 10 ^{ - 12} $ at $ 450~{\rm
pHz} $ with a sensitivity dropping approximately quadratically with frequency
until $ 10~{\rm pHz}$. Our search method opens a new frequency range for
gravitational wave detection and has profound implications for astrophysics,
cosmology, and particle physics.
