  We report on the linear optical properties of the chiral magnet Cu2OSeO3,
specifically associated with the absence of inversion symmetry, the chiral
crystallographic structure, and magnetic order. Through spectroscopic
ellipsometry, we observe local crystal-field excitations below the
charge-transfer gap. These crystal-field excitations are optically allowed due
to the lack of inversion symmetry at the Cu sites. Optical polarization
rotation measurements were used to study the structural chirality and magnetic
order. The temperature dependence of the natural optical rotation, originating
in the chiral crystal structure, provides evidence for a finite
magneto-electric effect in the helimagnetic phase. We find a large
magneto-optical susceptibility on the order of V(540nm)~10^4 rad/(T*m) in the
helimagnetic phase and a maximum Faraday rotation of ~165deg/mm in the
ferrimagnetic phase. The large value of V can be explained by considering spin
cluster formation and the relative ease of domain reorientation in this
metamagnetic material. The magneto-optical activity allows us to map the
magnetic phase diagram, including the skyrmion lattice phase. In addition to
this, we probe and discuss the nature of the various magnetic phase transitions
in Cu2OSeO3.
