  Spin qubits offer one of the most promising routes to the implementation of
quantum computers. Very recent results in semiconductor quantum dots show that
electrically-controlled gating schemes are particularly well-suited for the
realization of a universal set of quantum logical gates. Scalability to a
larger number of qubits, however, remains an issue for such semiconductor
quantum dots. In contrast, a chemical bottom-up approach allows one to produce
identical units in which localized spins represent the qubits. Molecular
magnetism has produced a wide range of systems with tailored properties, but
molecules permitting electrical gating have been lacking. Here we propose to
use the polyoxometalate [PMo12O40(VO)2]q-, where two localized spins-1/2 can be
coupled through the electrons of the central core. Via electrical manipulation
of the molecular redox potential, the charge of the core can be changed. With
this setup, two-qubit gates and qubit readout can be implemented.
