  We present the results of an X-ray spectral analysis of 153 galaxy clusters
observed with the Chandra, XMM-Newton, and Suzaku space telescopes. These
clusters, which span 0 < z < 1.5, were drawn from a larger, mass-selected
sample of galaxy clusters discovered in the 2500 square degree South Pole
Telescope Sunyaev Zel'dovich (SPT-SZ) survey. With a total combined exposure
time of 9.1 Ms, these data yield the strongest constraints to date on the
evolution of the metal content of the intracluster medium (ICM). We find no
evidence for strong evolution in the global (r<R500) ICM metallicity (dZ/dz =
-0.06 +/- 0.04 Zsun), with a mean value at z=0.6 of <Z> = 0.23 +/- 0.01 Zsun
and a scatter of 0.08 +/- 0.01 Zsun. These results imply that >60% of the
metals in the ICM were already in place at z=1 (at 95% confidence), consistent
with the picture of an early (z>1) enrichment. We find, in agreement with
previous works, a significantly higher mean value for the metallicity in the
centers of cool core clusters versus non-cool core clusters. We find weak
evidence for evolution in the central metallicity of cool core clusters (dZ/dz
= -0.21 +/- 0.11 Zsun), which is sufficient to account for this enhanced
central metallicity over the past ~10 Gyr. We find no evidence for metallicity
evolution outside of the core (dZ/dz = -0.03 +/- 0.06 Zsun), and no significant
difference in the core-excised metallicity between cool core and non-cool core
clusters. This suggests that strong radio-mode AGN feedback does not
significantly alter the distribution of metals at r>0.15R500. Given the
limitations of current-generation X-ray telescopes in constraining the ICM
metallicity at z>1, significant improvements on this work will likely require
next-generation X-ray missions.
