  We report a Raman scattering study of the pressure-induced collapse of the
Mott-like phases of Ca_3Ru_2O_7 (T_N=56 K) and Ca_2RuO_4 (T_N=110 K). The
pressure-dependence of the phonon and two-magnon excitations in these materials
indicate: (i) a pressure-induced collapse of the antiferromagnetic (AF)
insulating phase above P* ~ 55 kbar in Ca_3Ru_2O_7 and P* ~ 5-10 kbar in
Ca_2RuO_4, reflecting the importance of Ru-O octahedral distortions in
stabilizing the AF insulating phase; and (ii) evidence for persistent AF
correlations above the critical pressure of Ca_2RuO_4, suggestive of phase
separation involving AF insulator and ferromagnetic metal phases.
