  The crystal structures of Ni$X_2$(pyz)$_2$ ($X$ = Cl (\textbf{1}), Br
(\textbf{2}), I (\textbf{3}) and NCS (\textbf{4})) were determined at 298~K by
synchrotron X-ray powder diffraction. All four compounds consist of
two-dimensional (2D) square arrays self-assembled from octahedral NiN$_4$$X_2$
units that are bridged by pyz ligands. The 2D layered motifs displayed by
\textbf{1}-\textbf{4} are relevant to bifluoride-bridged
[Ni(HF$_2$)(pyz)$_2$]$Z$F$_6$ ($Z$ = P, Sb) which also possess the same 2D
layers. In contrast, terminal $X$ ligands occupy axial positions in
\textbf{1}-\textbf{4} and cause a staggering of adjacent layers. Long-range
antiferromagnetic order occurs below 1.5 (Cl), 1.9 (Br and NCS) and 2.5~K (I)
as determined by heat capacity and muon-spin relaxation. The single-ion
anisotropy and $g$ factor of \textbf{2}, \textbf{3} and \textbf{4} are measured
by electron spin resonance where no zero--field splitting was found. The
magnetism of \textbf{1}-\textbf{4} crosses a spectrum from
quasi-two-dimensional to three-dimensional antiferromagnetism. An excellent
agreement was found between the pulsed-field magnetization, magnetic
susceptibility and $T_\textrm{N}$ of \textbf{2} and \textbf{4}. Magnetization
curves for \textbf{2} and \textbf{4} calculated by quantum Monte Carlo
simulation also show excellent agreement with the pulsed-field data. \textbf{3}
is characterized as a three-dimensional antiferromagnet with the interlayer
interaction ($J_\perp$) slightly stronger than the interaction within the
two-dimensional [Ni(pyz)$_2$]$^{2+}$ square planes ($J_\textrm{pyz}$).
