  Quantum control is concerned with active manipulation of physical and
chemical processes on the atomic and molecular scale. This work presents a
perspective of progress in the field of control over quantum phenomena, tracing
the evolution of theoretical concepts and experimental methods from early
developments to the most recent advances. The current experimental successes
would be impossible without the development of intense femtosecond laser
sources and pulse shapers. The two most critical theoretical insights were (1)
realizing that ultrafast atomic and molecular dynamics can be controlled via
manipulation of quantum interferences and (2) understanding that optimally
shaped ultrafast laser pulses are the most effective means for producing the
desired quantum interference patterns in the controlled system. Finally, these
theoretical and experimental advances were brought together by the crucial
concept of adaptive feedback control, which is a laboratory procedure employing
measurement-driven, closed-loop optimization to identify the best shapes of
femtosecond laser control pulses for steering quantum dynamics towards the
desired objective. Optimization in adaptive feedback control experiments is
guided by a learning algorithm, with stochastic methods proving to be
especially effective. Adaptive feedback control of quantum phenomena has found
numerous applications in many areas of the physical and chemical sciences, and
this paper reviews the extensive experiments. Other subjects discussed include
quantum optimal control theory, quantum control landscapes, the role of
theoretical control designs in experimental realizations, and real-time quantum
feedback control. The paper concludes with a prospective of open research
directions that are likely to attract significant attention in the future.
