  The angular momentum of molecules, or, equivalently, their rotation in
three-dimensional space, is ideally suited for quantum control. Molecular
angular momentum is naturally quantized, time evolution is governed by a
well-known Hamiltonian with only a few accurately known parameters, and
transitions between rotational levels can be driven by external fields from
various parts of the electromagnetic spectrum. Control over the rotational
motion can be exerted in one-, two- and many-body scenarios, thereby allowing
to probe Anderson localization, target stereoselectivity of bimolecular
reactions, or encode quantum information, to name just a few examples. The
corresponding approaches to quantum control are pursued within separate, and
typically disjoint, subfields of physics, including ultrafast science, cold
collisions, ultracold gases, quantum information science, and condensed matter
physics. It is the purpose of this review to present the various control
phenomena, which all rely on the same underlying physics, within a unified
framework. To this end, we recall the Hamiltonian for free rotations, assuming
the rigid rotor approximation to be valid, and summarize the different ways for
a rotor to interact with external electromagnetic fields. These interactions
can be exploited for control --- from achieving alignment, orientation, or
laser cooling in a one-body framework, steering bimolecular collisions, or
realizing a quantum computer or quantum simulator in the many-body setting.
