  Herein, we show that single molecules containing multiple optical cycling
centers (CaO moieties) can exhibit superradiant phenomena. We demonstrate the
accuracy of the Frenkel exciton model at describing these superradiant states
via comparisons to high-level electronic structure methods. We then rationally
design molecules with superradiant properties optimized for laser cooling.
Lastly, we demonstrate how multi-photon superradiant phenomena can occur in
these novel molecular systems.
