  The nature of Fermi surface defines the physical properties of conductors and
many physical phenomena can be traced to its shape. Although the recent
discovery of a current-dependent nonlinear magnetoresistance in spin-polarized
non-magnetic materials has attracted considerable attention in spintronics,
correlations between this phenomenon and the underlying fermiology remain
unexplored. Here, we report the observation of nonlinear magnetoresistance at
room temperature in a semimetal WTe2, with an interesting temperature-driven
inversion. Theoretical calculations reproduce the nonlinear transport
measurements and allow us to attribute the inversion to temperature-induced
changes in Fermi surface convexity. We also report a large anisotropy of
nonlinear magnetoresistance in WTe2, due to its low symmetry of Fermi surfaces.
The good agreement between experiments and theoretical modeling reveals the
critical role of Fermi surface topology and convexity on the nonlinear
magneto-response. These results lay a new path to explore ramifications of
distinct fermiology for nonlinear transport in condensed-matter.
