  Dzyaloshinskii-Moriya interaction (DMI) is vital to form various chiral spin
textures, novel behaviors of magnons and permits their potential applications
in energy-efficient spintronic devices. Here, we realize a sizable bulk DMI in
a transition metal dichalcogenide (TMD) 2H-TaS2 by intercalating Fe atoms,
which form the chiral supercells with broken spatial inversion symmetry and
also act as the source of magnetic orderings. Using a newly developed protonic
gate technology, gate-controlled protons intercalation could further change the
carrier density and intensely tune DMI via the Ruderman-Kittel-Kasuya-Yosida
mechanism. The resultant giant topological Hall resistivity of 1.4 uohm.cm at
-5.2V (about 460% of the zero-bias value) is larger than most of the known
magnetic materials. Theoretical analysis indicates that such a large
topological Hall effect originates from the two-dimensional Bloch-type chiral
spin textures stabilized by DMI, while the large anomalous Hall effect comes
from the gapped Dirac nodal lines by spin-orbit interaction. Dual-intercalation
in 2HTaS2 provides a model system to reveal the nature of DMI in the large
family of TMDs and a promising way of gate tuning of DMI, which further enables
an electrical control of the chiral spin textures and related electromagnetic
phenomena.
