  From first-principles calculations, we predict that a single ethylene
molecule can form a stable complex with two transition metals (TM) such as Ti.
The resulting TM-ethylene complex then absorbs up to ten hydrogen molecules,
reaching to gravimetric storage capacity of 14 wt%. Dimerization,
polymerizations and incorporation of the TM-ethylene complexes in nanoporous
carbon materials have been also discussed. Our results are quite remarkable and
open a new approach to high-capacity hydrogen storage materials discovery.
