  Coherent control of bound state processes via the interfering overlapping
resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is
developed to control intramolecular vibrational redistribution (IVR). The
approach is applied to the flow of population between bonds in a model of
chaotic OCS vibrational dynamics, showing the ability to significantly alter
the extent and rate of IVR by varying quantum interference contributions.
