  Linear response approach to the relativistic coupled-cluster (RCC) theory has
been extended to estimate contributions from the parity and time-reversal
violating pseudoscalar-scalar (Ps-S) and scalar-pseudoscalar (S-Ps)
electron-nucleus interactions along with electric dipole moments (EDMs) of
electrons ($d_e$) interacting with internal electric and magnetic fields.
Random phase approximation (RPA) is also employed to produce results to compare
with the earlier reported values and demonstrate importance of the non-RPA
contributions arising through the RCC method. It shows that contributions from
the S-Ps interactions and $d_e$ arising through the hyperfine-induced effects
are very sensitive to the contributions from the high-lying virtual orbitals.
Combining atomic results with the nuclear shell-model calculations, we impose
constraints on the pion-nucleon coupling coefficients, and EDMs of proton and
neutron. These results are further used to constrain EDMs and chromo-EDMs of
up- and down-quarks by analyzing particle physics models.
