  Recent investigations have advanced the understanding of how
structure-property relationships in ferromagnetic metal alloys affect the
magnetization dynamics on nanosecond time-scales. A similar understanding for
magnetization dynamics on femto- to pico-second time-scales does not yet exist.
To address this, we perform time-resolved magneto optic Kerr effect (TRMOKE)
measurements of magnetization dynamics in Co-Fe alloys on femto- to nano-second
regimes. We show that Co-Fe compositions that exhibit low Gilbert damping
parameters also feature prolonged ultrafast demagnetization upon
photoexcitation. We analyze our experimental TR-MOKE data with the
three-temperature-model (3TM) and the Landau-Lifshitz-Gilbert equation. These
analyses reveal a strong compositional dependence of the dynamics across all
time-scales on the strength of electron-phonon interactions. Our findings are
beneficial to the spintronics and magnonics community, and will aid in the
quest for energy-efficient magnetic storage applications.
