  We discuss the abundances of interstellar CH, CH+, and CN in the Magellanic
Clouds (MC), derived from spectra of 7 SMC and 13 LMC stars obtained (mostly)
with the VLT/UVES. CH and/or CH+ are detected toward 3 SMC and 9 LMC stars; CN
is detected toward 2 stars. In the MC, the CH/H2 ratio is comparable to that
found for diffuse Galactic molecular clouds in some sight lines, but is lower
by factors up to 10-15 in others. The abundance of CH in the MC thus appears to
depend on local physical conditions -- and not just on metallicity. The
observed relationships between the column density of CH and those of CN, CH+,
Na I, and K I in the MC are generally consistent with the trends observed in
our Galaxy. Using existing data for the rotational populations of H2, we
estimate temperatures, radiation field strengths, and local hydrogen densities
for the diffuse molecular gas. Densities estimated from N(CH), assuming that CH
is produced via steady-state gas-phase reactions, are considerably higher; much
better agreement is found by assuming that the CH is made via the (still
undetermined) process(es) responsible for the observed CH+. The UVES spectra
also reveal absorption from the diffuse interstellar bands at 5780, 5797, and
6284 A in the MC. On average, the three DIBs are weaker by factors of 7-9 (LMC)
and about 20 (SMC), compared to those observed in Galactic sight lines with
similar N(H I), and by factors of order 2-6, relative to E(B-V), N(Na I), and
N(K I). The detection of several of the ``C2 DIBs'', with strengths similar to
those in comparable Galactic sight lines, however, indicates that no single,
uniform scaling factor (e.g., one related to metallicity) applies to all DIBs
(or all sight lines) in the MC. (abstract abridged)
