  Topological insulators constitute a new and fascinating class of matter with
insulating bulk yet metallic surfaces that host highly mobile charge carriers
with spin-momentum locking. Remarkably, the direction and magnitude of surface
currents can be controlled with tailored light beams, but the underlying
mechanisms are not yet well understood. To directly resolve the "birth" of such
photocurrents we need to boost the time resolution to the scale of elementary
scattering events ($\sim$ 10 fs). Here, we excite and measure photocurrents in
the three-dimensional model topological insulator $\mathrm{Bi}_2\mathrm{Se}_3$
with a time resolution as short as 20 fs by sampling the concomitantly emitted
broadband THz electromagnetic field from 1 to 40 THz. Remarkably, the ultrafast
surface current response is dominated by a charge transfer along the Se-Bi
bonds. In contrast, photon-helicity-dependent photocurrents are found to have
orders of magnitude smaller magnitude than expected from generation scenarios
based on asymmetric depopulation of the Dirac cone. Our findings are also of
direct relevance for optoelectronic devices based on topological-insulator
surface currents.
