  We employ interactions from chiral effective field theory and compute the
binding energies and low-lying excitations of calcium isotopes with the
coupled-cluster method. Effects of three-nucleon forces are included
phenomenologically as in-medium two-nucleon interactions, and the coupling to
the particle continuum is taken into account using a Berggren basis. The
computed ground-state energies and the low-lying 2+ states for the isotopes
42,48,50,52Ca are in good agreement with data, and we predict the excitation
energy of the first 2+ state in 54Ca at 1.9 MeV, displaying only a weak
sub-shell closure. In the odd-mass nuclei 53,55,61Ca we find that the positive
parity states deviate strongly from the naive shell model.
