  We use Raman scattering to study spin, charge, and lattice dynamics in
various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by
Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the
electron-phonon interaction strength, (2) an increased temperature-dependence
of the two-magnon energy and linewidth in the antiferromagnetic insulating
phase, and (3) evidence for charge gap development, and hysteresis associated
with the structural phase change, both of which are indicative of a first-order
metal-insulator transition (T_{MI}) and a coexistence of metallic and
insulating components for T < T_{MI}.
