  We use transport and neutron-scattering measurements to show that a
magnetic-field-induced transition from noncollinear to collinear spin
arrangement in adjacent CuO_{2} planes of lightly electron-doped
Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4} (x=0.01) crystals affects significantly both
the in-plane and out-of-plane resistivity. In the high-field collinear state,
the magnetoresistance (MR) does not saturate, but exhibits an intriguing
four-fold-symmetric angular dependence, oscillating from being positive at
B//[100] to being negative at B//[110]. The observed MR of more than 30% at low
temperatures induced by a modest modification of the spin structure indicates
an unexpectedly strong spin-charge coupling in electron-doped cuprates.
