new

Get trending papers in your email inbox!

Subscribe

Daily Papers

byAK and the research community

Dec 10

Atmospheric Transport Modeling of CO_2 with Neural Networks

Accurately describing the distribution of CO_2 in the atmosphere with atmospheric tracer transport models is essential for greenhouse gas monitoring and verification support systems to aid implementation of international climate agreements. Large deep neural networks are poised to revolutionize weather prediction, which requires 3D modeling of the atmosphere. While similar in this regard, atmospheric transport modeling is subject to new challenges. Both, stable predictions for longer time horizons and mass conservation throughout need to be achieved, while IO plays a larger role compared to computational costs. In this study we explore four different deep neural networks (UNet, GraphCast, Spherical Fourier Neural Operator and SwinTransformer) which have proven as state-of-the-art in weather prediction to assess their usefulness for atmospheric tracer transport modeling. For this, we assemble the CarbonBench dataset, a systematic benchmark tailored for machine learning emulators of Eulerian atmospheric transport. Through architectural adjustments, we decouple the performance of our emulators from the distribution shift caused by a steady rise in atmospheric CO_2. More specifically, we center CO_2 input fields to zero mean and then use an explicit flux scheme and a mass fixer to assure mass balance. This design enables stable and mass conserving transport for over 6 months with all four neural network architectures. In our study, the SwinTransformer displays particularly strong emulation skill (90-day R^2 > 0.99), with physically plausible emulation even for forward runs of multiple years. This work paves the way forward towards high resolution forward and inverse modeling of inert trace gases with neural networks.

  • 6 authors
·
Aug 20, 2024

Optimizing Methane Detection On Board Satellites: Speed, Accuracy, and Low-Power Solutions for Resource-Constrained Hardware

Methane is a potent greenhouse gas, and detecting its leaks early via hyperspectral satellite imagery can help mitigate climate change. Meanwhile, many existing missions operate in manual tasking regimes only, thus missing potential events of interest. To overcome slow downlink rates cost-effectively, onboard detection is a viable solution. However, traditional methane enhancement methods are too computationally demanding for resource-limited onboard hardware. This work accelerates methane detection by focusing on efficient, low-power algorithms. We test fast target detection methods (ACE, CEM) that have not been previously used for methane detection and propose a Mag1c-SAS - a significantly faster variant of the current state-of-the-art algorithm for methane detection: Mag1c. To explore their true detection potential, we integrate them with a machine learning model (U-Net, LinkNet). Our results identify two promising candidates (Mag1c-SAS and CEM), both acceptably accurate for the detection of strong plumes and computationally efficient enough for onboard deployment: one optimized more for accuracy, the other more for speed, achieving up to ~100x and ~230x faster computation than original Mag1c on resource-limited hardware. Additionally, we propose and evaluate three band selection strategies. One of them can outperform the method traditionally used in the field while using fewer channels, leading to even faster processing without compromising accuracy. This research lays the foundation for future advancements in onboard methane detection with minimal hardware requirements, improving timely data delivery. The produced code, data, and models are open-sourced and can be accessed from https://github.com/zaitra/methane-filters-benchmark.

  • 3 authors
·
Jul 2

Characterising the Atmosphere of 55 Cancri e: 1D Forward Model Grid for Current and Future JWST Observations

Recent JWST observations with NIRCam and MIRI of the ultra-short-period super-Earth 55 Cancri e indicate a possible volatile atmosphere surrounding the planet. Previous analysis of the NIRCam spectra suggested potential absorption features from CO2 or CO and significant sub-weekly variability. The MIRI low-resolution spectrum does not contain substantial features but was found to be consistent with effective heat redistribution models. In this work, we computed a grid of over 25000 self-consistent 1D forward models incorporating H-N-O-C-S-P-Si-Ti equilibrium chemistry and assessed plausible atmospheric compositions based on the current JWST data. Despite exhaustive analysis, the composition and properties of the atmosphere remain elusive. While our results statistically favour a global, hydrogen-free, nitrogen-dominated atmosphere enriched in PO and CO2, various alternative compositions, including H2O-,CO-, PH3-, or Si-bearing remain viable explanations. Unconstrained heat redistribution efficiency and absolute NIRCam flux are among the largest sources of uncertainty in our analysis. We also find that the heat redistribution factor and surface pressure are highly degenerate with atmospheric composition, and that these parameters cannot be independently constrained using current JWST observations. Furthermore, we show that the observed variability may arise from dynamic interactions between the atmosphere and an underlying magma ocean, driving rapid shifts in atmospheric chemistry and thermal emission. Our results highlight the importance of using self-consistent forward models when analysing novel JWST spectra with limited signal-to-noise ratios -- such as those of 55 Cancri e -- as it allows for a more comprehensive evaluation of potential atmospheric scenarios while also being less sensitive to subtle spectral differences than retrievals...

  • 12 authors
·
Mar 20

PDRs4All. XII. FUV-driven formation of hydrocarbon radicals and their relation with PAHs

We present subarcsecond-resolution ALMA mosaics of the Orion Bar PDR in [CI] 609 um, C2H (4-3), and C18O (3-2) emission lines, complemented by JWST images of H2 and aromatic infrared band (AIB) emission. The rim of the Bar shows very corrugated structures made of small-scale H2 dissociation fronts (DFs). The [CI] 609 um emission peaks very close (~0.002 pc) to the main H2-emitting DFs, suggesting the presence of gas density gradients. These DFs are also bright and remarkably similar in C2H emission, which traces 'hydrocarbon radical peaks' characterized by very high C2H abundances, reaching up to several x10^-7. The high abundance of C2H and of related hydrocarbon radicals, such as CH3, CH2, and CH, can be attributed to gas-phase reactions driven by elevated temperatures, the presence of C+ and C, and the reactivity of FUV-pumped H2. The hydrocarbon radical peaks roughly coincide with maxima of the 3.4/3.3 um AIB intensity ratio, a proxy for the aliphatic-to-aromatic content of PAHs. This implies that the conditions triggering the formation of simple hydrocarbons also favor the formation (and survival) of PAHs with aliphatic side groups, potentially via the contribution of bottom-up processes in which abundant hydrocarbon radicals react in situ with PAHs. Ahead of the DFs, in the atomic PDR zone (where [H]>>[H2]), the AIB emission is brightest, but small PAHs and carbonaceous grains undergo photo-processing due to the stronger FUV field. Our detection of trace amounts of C2H in this zone may result from the photoerosion of these species. This study provides a spatially resolved view of the chemical stratification of key carbon carriers in a PDR. Overall, both bottom-up and top-down processes appear to link simple hydrocarbon molecules with PAHs in molecular clouds; however, the exact chemical pathways and their relative contributions remain to be quantified.

  • 28 authors
·
Mar 5

Gas dynamics around a Jupiter mass planet: II. Chemical evolution of circumplanetary material

In an ongoing effort to understand planet formation the link between the chemistry of the protoplanetary disk and the properties of resulting planets have long been a subject of interest. These connections have generally been made between mature planets and young protoplanetary disks through the carbon-to-oxygen (C/O) ratio. In a rare number of systems, young protoplanets have been found within their natal protoplanetary disks. These systems offer a unique opportunity to directly study the delivery of gas from the protoplanetary disk to the planet. In this work we post-process 3D numerical simulations of an embedded Jupiter-massed planet in its protoplanetary disk to explore the chemical evolution of gas as it flows from the disk to the planet. The relevant dust to this chemical evolution is assumed to be small, co-moving grains with a reduced dust-to-gas ratio indicative of the upper atmosphere of a protoplanetary disk. We find that as the gas enters deep into the planet's gravitational well, it warms significantly (up to sim 800 K), releasing all of the volatile content from the ice phase. This change in phase can influence our understanding of the delivery of volatile species to the atmospheres of giant planets. The primary carbon, oxygen, and sulfur carrying ices: CO_2, H_2O, and H_2S are released into the gas phase and along with the warm gas temperatures near the embedded planets lead to the production of unique species like CS, SO, and SO_2 compared to the protoplanetary disk. We compute the column densities of SO, SO_2, CS, and H_2CS in our model and find that their values are consistent with previous observational studies.

  • 3 authors
·
Nov 26, 2024

First detections of CO absorption in the Magellanic Clouds and direct measurement of the CO-to-H_2 ratio

Molecular hydrogen (H_2) is by far the most abundant molecule in the Universe. However, due to the low emissivity of H_2, carbon monoxide (CO) is widely used instead to trace molecular gas in galaxies. The relative abundances of these molecules is expected to depend on both physical (e.g., density) and chemical (e.g., metal enrichment) properties of the gas, making direct measurements in diverse environments crucial. We present a systematic search for CO in absorption toward 34 stars behind H_2 gas in the Magellanic Clouds using the Hubble Space Telescope. We report the first two definitive detections of CO absorption in the Large Magellanic Cloud (LMC) and one in the Small Magellanic Cloud (SMC), along with stringent upper limits for the remaining sightlines. Non-detections of CO are consistent with models of low thermal pressures and/or low metallicities while detections at the lower metallicities of the Magellanic Clouds require higher thermal pressures, P_{rm th}=10^5-10^6,K,cm^{-3} than detections the Milky Way at similar N({rm H_2}). Notably, the high density derived from the rotational excitation of CO towards SK,143 in the SMC suggests full molecularization of CO in the absorbing cloud, with CO/H_2 = 8.3^{+2.0}_{-1.6}times10^{-5} consistent with the standard ratio (3.2times10^{-4}) measured in dense molecular gas in the Milky Way, scaled to the SMC's 0.2,Z_{odot} metallicity.

  • 3 authors
·
Mar 16

ACE2-SOM: Coupling to a slab ocean and learning the sensitivity of climate to changes in CO_2

While autoregressive machine-learning-based emulators have been trained to produce stable and accurate rollouts in the climate of the present-day and recent past, none so far have been trained to emulate the sensitivity of climate to substantial changes in CO_2 or other greenhouse gases. As an initial step we couple the Ai2 Climate Emulator version 2 to a slab ocean model (hereafter ACE2-SOM) and train it on output from a collection of equilibrium-climate physics-based reference simulations with varying levels of CO_2. We test it in equilibrium and non-equilibrium climate scenarios with CO_2 concentrations seen and unseen in training. ACE2-SOM performs well in equilibrium-climate inference with both in-sample and out-of-sample CO_2 concentrations, accurately reproducing the emergent time-mean spatial patterns of surface temperature and precipitation change with CO_2 doubling, tripling, or quadrupling. In addition, the vertical profile of atmospheric warming and change in extreme precipitation rates with increased CO_2 closely agree with the reference model. Non-equilibrium-climate inference is more challenging. With CO_2 increasing gradually at a rate of 2% year^{-1}, ACE2-SOM can accurately emulate the global annual mean trends of surface and lower-to-middle atmosphere fields but produces unphysical jumps in stratospheric fields. With an abrupt quadrupling of CO_2, ML-controlled fields transition unrealistically quickly to the 4xCO_2 regime. In doing so they violate global energy conservation and exhibit unphysical sensitivities of and surface and top of atmosphere radiative fluxes to instantaneous changes in CO_2. Future emulator development needed to address these issues should improve its generalizability to diverse climate change scenarios.

  • 9 authors
·
Dec 5, 2024

Pre-perihelion Development of Interstellar Comet 3I/ATLAS

We describe pre-perihelion optical observations of interstellar comet 3I/ATLAS taken during July - September 2025 using the Nordic Optical Telescope. Fixed aperture photometry of the comet is well described by a power law function of heliocentric distance, rH, with the exponent (``index") n = 3.8+/-0.3 across the 4.6 au to 1.8 au distance range (phase function 0.04+/-0.02 magnitude/degree assumed). This indicates that the dust production rates vary in proportion to rH**(-1.8+/-0.3). An rH**(-2) variation is expected of a strongly volatile material, and consistent with independent spectroscopic observations showing that carbon dioxide is the primary driver of activity. The measured heliocentric index is unremarkable in the context of solar system comets, for which n is widely dispersed, and provides no basis on which to describe 3I as either dynamically old (thermally processed) or new (pristine). The morphology of the comet changes from a Sun-facing dust fan in the early 2025 July observations, to one dominated by an antisolar dust tail at later dates. We attribute the delayed emergence of the tail to the large size (effective radius 0.1 mm) and slow ejection (5 m/s) of the optically dominant dust particles, and their consequently sluggish response to solar radiation pressure. Small (micron-sized) particles may be present but not in numbers sufficient to dominate the scattering cross-section. Their relative depletion possibly reflects interparticle cohesion, which binds small particles more effectively than large ones. A similar preponderance of 0.1 mm grains was reported in 2I/Borisov. However, 2I differed from 3I in having a much smaller (asteroid-like) heliocentric index, n = 1.9+/-0.1. Dust production rates in 3I are 180 kg/s at 2 au, compared with 70 kg/s in 2I/Borisov at the same distance.

  • 2 authors
·
Oct 21

The chemical inventory of the planet-hosting disk PDS 70

As host to two accreting planets, PDS 70 provides a unique opportunity to probe the chemical complexity of atmosphere-forming material. We present ALMA Band 6 observations of the PDS~70 disk and report the first chemical inventory of the system. With a spatial resolution of 0.4''-0.5'' (sim50 au), 12 species are detected, including CO isotopologues and formaldehyde, small hydrocarbons, HCN and HCO+ isotopologues, and S-bearing molecules. SO and CH3OH are not detected. All lines show a large cavity at the center of the disk, indicative of the deep gap carved by the massive planets. The radial profiles of the line emission are compared to the (sub-)mm continuum and infrared scattered light intensity profiles. Different molecular transitions peak at different radii, revealing the complex interplay between density, temperature and chemistry in setting molecular abundances. Column densities and optical depth profiles are derived for all detected molecules, and upper limits obtained for the non detections. Excitation temperature is obtained for H2CO. Deuteration and nitrogen fractionation profiles from the hydro-cyanide lines show radially increasing fractionation levels. Comparison of the disk chemical inventory to grids of chemical models from the literature strongly suggests a disk molecular layer hosting a carbon to oxygen ratio C/O>1, thus providing for the first time compelling evidence of planets actively accreting high C/O ratio gas at present time.

  • 6 authors
·
Jan 20, 2021